# Publications

2021
Golja, C. M., L. W. Chew, J. A. Dykema, and D. W. Keith. “Aerosol Dynamics in the Near Field of the SCoPEx Stratospheric Balloon Experiment.” Journal of Geophysical Research (2021). Publisher's VersionAbstract
Stratospheric aerosol injection (SAI) might alleviate some climate risks associated with accumulating greenhouse gases. Reduction of specific process uncertainties relevant to the distribution of aerosol in a turbulent stratospheric wake is necessary to support informed decisions about aircraft deployment of this technology. To predict aerosol size distributions we apply microphysical parameterizations of nucleation, condensation and coagulation to simulate an aerosol plume generated via injection of calcite powder or sulphate into a stratospheric wake with velocity and turbulence simulated by a three‐dimensional (3D) fluid dynamic calculation. We apply the model to predict the aerosol distribution that would be generated by a propeller wake in the Stratospheric Controlled Perturbation Experiment (SCoPEx). We find that injecting 0.1 g s‐1 calcite aerosol produces a nearly monodisperse plume and that at the same injection rate, condensable sulphate aerosol forms particles with average radii of 0.1 µm at 3 km downstream. We test the sensitivity of plume aerosol composition, size, and optical depth to the mass injection rate and injection location. Aerosol size distribution depends more strongly on injection rate than injection configuration. Comparing plume properties with specifications of a typical photometer, we find that plumes could be detected optically as the payload flies under the plume. These findings test the relevance of in situ sampling of aerosol properties by the SCoPEx outdoor experiment to enable quantitative tests of microphysics in a stratospheric plume. Our findings provide a basis for developing predictive models of SAI using aerosols formed in stratospheric aircraft wakes.
Seeley, Jacob T., Nicholas J. Lutsko, and David W. Keith. “Designing a radiative antidote to CO2.” Geophysical Research Letters (2021). Publisher's VersionAbstract
Solar Radiation Modification (SRM) reduces the CO2‐induced change to the mean global hydrological cycle disproportionately more than it reduces the CO2‐induced increase in mean surface temperature. Thus if SRM were used to offset all CO2‐induced mean warming, global‐mean precipitation would be less than in an unperturbed climate. Here we show that the mismatch between the mean hydrological effects of CO2 and SRM may partly be alleviated by spectrally tuning the SRM intervention (reducing insolation at some wavelengths more than others). By concentrating solar dimming at near‐infrared wavelengths, where H2O has strong absorption bands, the direct effect of CO2 on the tropospheric energy budget can be offset, which minimizes perturbations to the mean hydrological cycle. Idealized cloud‐resolving simulations of radiative‐convective equilibrium confirm that spectrally‐tuned SRM can simultaneously maintain mean surface temperature and precipitation at their unperturbed values even as large quantities of CO2 are added to the atmosphere.
2020
Reynolds, Jesse, and Joshua Horton. “An earth system governance perspective on solar geoengineering.” Earth System Governance 3 (2020). Publisher's VersionAbstract
Solar geoengineering appears capable of reducing climate change and the associated risks. In part because it would be global in effect, the governance of solar geoengineering is a central concern. The Earth System Governance (ESG) Project includes many researchers who, to varying degrees, utilize a common vocabulary and research framework. Despite the clear mutual relevance of solar geoengineering and ESG, few ESG researchers have considered the topic in substantial depth. To stimulate its sustained uptake as a subject within the ESG research program, we identify significant contributions thus far by ESG scholars on the subject of solar geoengineering governance and survey the wider solar geoengineering governance literature from the perspective of the new ESG research framework. Based on this analysis, we also suggest specific potential lines of inquiry that we believe are ripe for research by ESG scholars: nonstate actors’ roles, polycentricity, public engagement and participation, and the Anthropocene.
Dai, Zhen, Debra K. Weisenstein, Frank N. Keutsch, and David W. Keith. “Experimental reaction rates constrain estimates of ozone response to calcium carbonate geoengineering.” Communications Earth & Environment 1, no. 63 (2020). Publisher's VersionAbstract
Stratospheric solar geoengineering (SG) would impact ozone by heterogeneous chemistry. Evaluating these risks and methods to reduce them will require both laboratory and modeling work. Prior model-only work showed that CaCO3 particles would reduce, or even reverse ozone depletion. We reduce uncertainties in ozone response to CaCO3 via experimental determination of uptake coefficients and model evaluation. Specifically, we measure uptake coefficients of HCl and HNO3 on CaCO3 as well as HNO3 and ClONO2 on CaCl2 at stratospheric temperatures using a flow tube setup and a flask experiment that determines cumulative long-term uptake of HCl on CaCO3. We find that particle ageing causes significant decreases in uptake coefficients on CaCO3. We model ozone response incorporating the experimental uptake coefficients in the AER-2D model. With our new empirical reaction model, the global mean ozone column is reduced by up to 3%, whereas the previous work predicted up to 27% increase for the same SG scenario. This result is robust under our experimental uncertainty and many other assumptions. We outline systematic uncertainties that remain and provide three examples of experiments that might further reduce uncertainties of CaCO3 SG. Finally, we highlight the importance of the link between experiments and models in studies of SG.
Reynolds, Jesse, and Joshua Horton. “An earth system governance perspective on solar geoengineering.” Earth System Governance 3 (2020). Publisher's VersionAbstract
Solar geoengineering appears capable of reducing climate change and the associated risks. In part because it would be global in effect, the governance of solar geoengineering is a central concern. The Earth System Governance (ESG) Project includes many researchers who, to varying degrees, utilize a common vocabulary and research framework. Despite the clear mutual relevance of solar geoengineering and ESG, few ESG researchers have considered the topic in substantial depth. To stimulate its sustained uptake as a subject within the ESG research program, we identify significant contributions thus far by ESG scholars on the subject of solar geoengineering governance and survey the wider solar geoengineering governance literature from the perspective of the new ESG research framework. Based on this analysis, we also suggest specific potential lines of inquiry that we believe are ripe for research by ESG scholars: nonstate actors’ roles, polycentricity, public engagement and participation, and the Anthropocene.
Reynolds, Jesse L., and Joshua B. Horton. “An earth system governance perspective on solar geoengineering.” Earth System Governance 3 (2020).Abstract
Solar geoengineering appears capable of reducing climate change and the associated risks. In part because it would be global in effect, the governance of solar geoengineering is a central concern. The Earth System Governance (ESG) Project includes many researchers who, to varying degrees, utilize a common vocabulary and research framework. Despite the clear mutual relevance of solar geoengineering and ESG, few ESG researchers have considered the topic in substantial depth. To stimulate its sustained uptake as a subject within the ESG research program, we identify significant contributions thus far by ESG scholars on the subject of solar geoengineering governance and survey the wider solar geoengineering governance literature from the perspective of the new ESG research framework. Based on this analysis, we also suggest specific potential lines of inquiry that we believe are ripe for research by ESG scholars: nonstate actors’ roles, polycentricity, public engagement and participation, and the Anthropocene.
Horton, Joshua B., and Barbara Koromenos. “Steering and Influence in Transnational Climate Governance: Nonstate Engagement in Solar Geoengineering Research.” Global Environmental Politics 20, no. 3 (2020): 93-111. Publisher's VersionAbstract
Theorists of transnational climate governance (TCG) seek to account for the increasing involvement of nonstate and substate actors in global climate policy. While transnational actors have been present in the emerging field of solar geoengineering—a novel technology intended to reflect a fraction of sunlight back to space to reduce climate impacts— many of their most significant activities, including knowledge dissemination, scientific capacity building, and conventional lobbying, are not captured by the TCG framework. Insofar as TCG is identified with transnational governance and transnational governance is important to reducing climate risks, an incomplete TCG framework is problematic for effective policy making. We attribute this shortcoming on the part of TCG to its exclusive focus on steering and corollary exclusion of influence as a critical component of governance. Exercising influence, for example, through inside and outside lobbying, is an important part of transnational governance—it complements direct governing with indirect efforts to inform, persuade, pressure, or otherwise influence both governor and governed. Based on an empirical analysis of solar geoengineering research governance and a theoretical consideration of alternative literatures, including research on interest groups and nonstate advocacy, we call for a broader theory of transnational governance that integrates steering and influence in a way that accounts for the full array of nonstate and substate engagements beyond the state.
Lutsko, Nicholas J., Jacob T. Seeley, and David W. Keith. “Estimating Impacts and Trade‐offs in Solar Geoengineering Scenarios With a Moist Energy Balance Model.” Geophysical Research Letters 47, no. 9 (2020). Publisher's VersionAbstract
There are large uncertainties in the potential impacts of solar radiation modification (SRM) and in how these impacts depend on the way SRM is deployed. One open question concerns trade‐offs between latitudinal profiles of insolation reduction and climate response. Here, a moist energy balance model is used to evaluate several SRM proposals, providing fundamental insight into how the insolation reduction profile affects the climate response. The optimal SRM profile is found to depend on the intensity of the intervention, as the most effective profile for moderate SRM focuses the reduction at high latitudes, whereas the most effective profile for strong SRM is tropically amplified. The effectiveness of SRM is also shown to depend on when it is applied, an important factor to consider when designing SRM proposals. Using an energy balance model allows us to provide physical explanations for these results while also suggesting future avenues of research with comprehensive climate models.
Horton, Joshua B., Penehuro Lefale, and David Keith. “Parametric Insurance for Solar Geoengineering: Insights from the Pacific Catastrophe Risk Assessment and Financing Initiative.” Global Policy, no. Special Issue (2020). Publisher's VersionAbstract
Solar geoengineering (SG) entails using technology to modify the Earth's radiative balance to offset some of the climate changes caused by long‐lived greenhouse gases. Parametric insurance, which delivers payouts when specific physical indices (such as wind speed) cross predefined thresholds, was recently proposed by two of us as a compensation mechanism for SG with the potential to ease disagreements about the technology and to facilitate cooperative deployment; we refer to this proposal as reduced‐rate climate risk insurance for solar geoengineering, or ‘RCG’. Here we probe the plausibility of RCG by exploring the Pacific Catastrophe Risk Assessment and Financing Initiative (PCRAFI), a sovereign risk pool providing parametric insurance coverage against tropical cyclones and earthquakes/tsunamis to Pacific island countries since 2013. Tracing the history of PCRAFI and considering regional views on insurance as compensation necessitates reconfiguring RCG in a way that shifts the focus away from bargaining between developed and developing countries toward bargaining among developed countries. This revised version of RCG is challenged by an assumption of broad developed country support for sovereign climate insurance in the developing world, but it also better reflects the underlying incentive structure and distribution of power.
Keith, David, and Peter Irvine. “Halving warming with stratospheric aerosol geoengineering moderates policy-relevant climate hazards.” Environmental Research Letters 15, no. 4 (2020). Publisher's VersionAbstract
Stratospheric aerosol geoengineering is a proposal to artificially thicken the layer of reflective aerosols in the stratosphere and it is hoped that this may offer a means of reducing average climate changes. However, previous work has shown that it could not perfectly offset the effects of climate change and there is a concern that it may worsen climate impacts in some regions. One approach to evaluating this concern is to test whether the absolute magnitude of climate change at each location is significantly increased (exacerbated) or decreased (moderated) relative to the period just preceding deployment. In prior work it was found that halving warming with an idealized solar constant reduction would substantially reduce climate change overall, exacerbating change in a small fraction of places. Here, we test if this result holds for a more realistic representation of stratospheric aerosol geoengineering using the data from the geoengineering large ensemble (GLENS). Using a linearized scaling of GLENS we find that halving warming with stratospheric aerosols moderates important climate hazards in almost all regions. Only 1.3% of land area sees exacerbation of change in water availability, and regions that are exacerbated see wetting not drying contradicting the common assumption that solar geoengineering leads to drying in general. These results suggest that halving warming with stratospheric aerosol geoengineering could potentially reduce key climate hazards substantially while avoiding some problems associated with fully offsetting warming.
2019
MacMartin, Douglas, Peter Irvine, Ben Kravitz, and Joshua Horton. “Technical characteristics of a solar geoengineering deployment and implications for governance.” Climate Policy 19, no. 10 (2019): 1325-1339. Publisher's VersionAbstract
Consideration of solar geoengineering as a potential response to climate change will demand complex decisions. These include not only the choice of whether to deploy solar engineering, but decisions regarding how to deploy, and ongoing decisionmaking throughout deployment. Research on the governance of solar geoengineering to date has primarily engaged only with the question of whether to deploy. We examine the science of solar geoengineering in order to clarify the technical dimensions of decisions about deployment – both strategic and operational – and how these might influence governance considerations, while consciously refraining from making specific recommendations. The focus here is on a hypothetical deployment rather than governance of the research itself. We first consider the complexity surrounding the design of a deployment scheme, in particular the complicated and difficult decision of what its objective(s) would be, given that different choices for how to deploy will lead to different climate outcomes. Next, we discuss the on-going decisions across multiple timescales, from the sub-annual to the multi-decadal. For example, feedback approaches might effectively manage some uncertainties, but would require frequent adjustments to the solar geoengineering deployment in response to observations. Other decisions would be tied to the inherently slow process of detection and attribution of climate effects in the presence of natural variability. Both of these present challenges to decision-making. These considerations point toward particular governance requirements, including an important role for technical experts – with all the challenges that entails.
Dagon, Katherine, and Daniel Schrag. “Quantifying the effects of solar geoengineering on vegetation.” Climatic Change 152, no. 1-2 (2019): 235–251. Publisher's VersionAbstract
Climate change will have significant impacts on vegetation and biodiversity. Solar geoengineering has potential to reduce the climate effects of greenhouse gas emissions through albedo modification, yet more research is needed to better understand how these techniques might impact terrestrial ecosystems. Here, we utilize the fully coupled version of the Community Earth System Model to run transient solar geoengineering simulations designed to stabilize radiative forcing starting mid-century, relative to the Representative Concentration Pathway 6 (RCP6) scenario. Using results from 100-year simulations, we analyze model output through the lens of ecosystem-relevant metrics. We find that solar geoengineering improves the conservation outlook under climate change, but there are still potential impacts on terrestrial vegetation. We show that rates of warming and the climate velocity of temperature are minimized globally under solar geoengineering by the end of the century, while trends persist over land in the Northern Hemisphere. Moisture is an additional constraint on vegetation, and in the tropics the climate velocity of precipitation dominates over that of temperature. Shifts in the amplitude of temperature and precipitation seasonal cycles have implications for vegetation phenology. Different metrics for vegetation productivity also show decreases under solar geoengineering relative to RCP6, but could be related to the model parameterization of nutrient cycling. The coupling of water and carbon cycles is found to be an important mechanism for understanding changes in ecosystems under solar geoengineering.
Burns, Lizzie, David Keith, Peter Irvine, and Joshua Horton. “Belfer Technology Factsheet Series: Solar Geoengineering” (2019).Abstract
Solar geoengineering refers to a set of emerging technologies that could alter the Earth’s radiative balance— perhaps through injecting aerosols into the stratosphere, where they would reflect a small fraction of sunlight back into space—reducing the amount of climate change caused by greenhouse gases. It could not replace reducing emissions (mitigation), coping with a changing climate (adaptation), or carbon dioxide removal (CDR). Yet it does have the potential to supplement these efforts, and it might provide reductions in climate risk that are unachievable by other means.
Keith, David, and Joshua Horton. “Multilateral parametric climate risk insurance: a tool to facilitate agreement about deployment of solar geoengineering?Climate Policy (2019). Publisher's VersionAbstract
States will disagree about deployment of solar geoengineering, technologies that would reflect a small portion of incoming sunlight to reduce risks of climate change, and most disagreements will be grounded in conflicting interests. States that object to deployment will have many options to oppose it, so states favouring deployment will have a powerful incentive to meet their objections. Objections rooted in opposition to the anticipated unequal consequences of deployment may be met through compensation, yet climate policy is inhospitable to compensation via liability. We propose that multilateral parametric climate risk insurance might be a useful tool to facilitate agreement on solar geoengineering deployment. With parametric insurance, predetermined payouts are triggered when climate indices deviate from set ranges. We suggest that states favouring deployment could underwrite reduced-rate parametric climate insurance. This mechanism would be particularly suited to resolving disagreements based on divergent judgments about the outcomes of proposed implementation. This would be especially relevant in cases where disagreements are rooted in varying levels of trust in climate model predictions of solar geoengineering effectiveness and risks. Negotiations over the pricing and terms of a parametric risk pool would make divergent judgments explicit and quantitative. Reduced-rate insurance would provide a way for states that favour implementation to demonstrate their confidence in solar geoengineering by underwriting risk transfer and ensuring compensation without the need for attribution. This would offer a powerful incentive for states opposing implementation to moderate their opposition.
Vattioni, Sandro, Debra Weisenstein, David Keith, Aryeh Feinberg, Thomas Peter, and Andrea Stenke. “Exploring accumulation-mode H2SO4 versus SO2 stratospheric sulfate geoengineering in a sectional aerosol–chemistry–climate model.” Atmospheric Chemistry and Physics 19 (2019). Publisher's VersionAbstract
Heyen, Daniel, Joshua Horton, and Juan Moreno-Cruz. “Strategic implications of counter-geoengineering: Clash or cooperation?Journal of Environmental Economics and Management 95 (2019): 153-177. Publisher's VersionAbstract
Solar geoengineering has received increasing attention as an option to temporarily stabilize global temperatures. A key concern is that heterogeneous preferences over the optimal amount of cooling combined with low deployment costs may allow the country with the strongest incentive for cooling, the so-called free-driver, to impose a substantial externality on the rest of the world. We analyze whether the threat of counter-geoengineering technologies capable of negating the climatic effects of solar geoengineering can overcome the free-driver problemand tilt the game in favour of international cooperation. Our game-theoreticalmodel of countries with asymmetric preferences allows for a rigorous analysis of the strategic interaction surrounding solar geoengineering and counter-geoengineering.We find that countergeoengineering prevents the free-driver outcome, but not always with benign effects. The presence of counter-geoengineering leads to either a climate clash where countries engage in a non-cooperative escalation of opposing climate interventions (negative welfare effect), a moratorium treaty where countries commit to abstain from either type of climate intervention (indeterminate welfare effect), or cooperative deployment of solar geoengineering (positivewelfare effect).We show that the outcome depends crucially on the degree of asymmetry in temperature preferences between countries.
Svoboda, Toby, Peter Irvine, Daniel Callies, and Masahiro Sugiyama. “The potential for climate engineering with stratospheric sulfate aerosol injections to reduce climate injustice.” Journal of Global Ethics (2019). Publisher's VersionAbstract
Climate engineering with stratospheric sulfate aerosol injections (SSAI) has the potential to reduce risks of injustice related to anthropogenic emissions of greenhouse gases. Relying on evidence from modeling studies, this paper makes the case that SSAI could have the potential to reduce many of the key physical risks of climate change identified by the Intergovernmental Panel on Climate Change. Such risks carry potential injustice because they are often imposed on low-emitters who do not benefit from climate change. Because SSAI has the potential to reduce those risks, it thereby has the potential to reduce the injustice associated with anthropogenic emissions. While acknowledging important caveats, including uncertainty in modeling studies and the potential for SSAI to carry its own risks of injustice, the paper argues that there is a strong case for continued research into SSAI, especially if attention is paid to how it might be used to reduce emissions-driven injustice.
Irvine, Peter, Kerry Emanuel, Jie He, Larry Horowitz, Gabriel Vecchi, and David Keith. “Halving warming with idealized solar geoengineering moderates key climate hazards.” Nature Climate Change (2019). Publisher's VersionAbstract

Solar geoengineering (SG) has the potential to restore average surface temperatures by increasing planetary albedo, but this could reduce precipitation. Thus, although SG might reduce globally aggregated risks, it may increase climate risks for some regions. Here, using the high-resolution forecastoriented low ocean resolution (HiFLOR) model—which resolves tropical cyclones and has an improved representation of present-day precipitation extremes—alongside 12 models from the Geoengineering Model Intercomparison Project (GeoMIP), we analyse the fraction of locations that see their local climate change exacerbated or moderated by SG. Rather than restoring temperatures, we assume that SG is applied to halve the warming produced by doubling CO2 (half-SG). In HiFLOR, half-SG offsets most of the CO2-induced increase of simulated tropical cyclone intensity. Moreover, none of temperature, water availability, extreme temperature or extreme precipitation are exacerbated under half-SG when averaged over any Intergovernmental Panel on Climate Change (IPCC) Special Report on Extremes (SREX) region. Indeed, for both extreme precipitation and water availability, less than 0.4% of the ice-free land surface sees exacerbation. Thus, while concerns about the inequality of solar geoengineering impacts are appropriate, the quantitative extent of inequality may be overstated.

2018
Horton, Joshua B.Parametric Insurance as an Alternative to Liability for Compensating Climate Harms.” Carbon & Climate Law Review 12, no. 4 (2018): 285-296. Publisher's VersionAbstract
Interstate compensation for climate change based on legal liability faces serious obstacles. Structural incongruities related to causation, time, scope, and scale impede application of tort law to climate change, while political opposition from developed countries prevents intergovernmental consideration of liability as a means of compensating for climate damages. Insurance, however, in particular parametric insurance triggered by objective environmental indices, is emerging as a promising alternative to liability. This is manifest in the UNFCCC and the Paris Agreement, which ruled out recourse to legal liability, and in the formation and expansion of regional sovereign climate risk insurance schemes in the Caribbean, Africa, and the Pacific. Theory and early practice suggest that parametric insurance exhibits five key advantages compared to legal liability in the climate change context: (1) it does not require that causation be demonstrated; (2) it has evolved to provide catastrophic coverage; (3) it is oriented toward the future rather than the past; (4) it is contractual, rather than adversarial, in nature; and (5) it provides a high degree of predictability. Compensation based on parametric insurance represents a novel climate policy option with significant potential to advance climate politics.
Smith, Wake, and Gernot Wagner. “Stratospheric aerosol injection tactics and costs in the first 15 years of deployment.” Environmental Research Letters 13 (2018). Publisher's VersionAbstract
We review the capabilities and costs of various lofting methods intended to deliver sulfates into the lower stratosphere. We lay out a future solar geoengineering deployment scenario of halving the increase in anthropogenic radiative forcing beginning 15 years hence, by deploying material to altitudes as high as ~20 km. After surveying an exhaustive list of potential deployment techniques, we settle upon an aircraft-based delivery system. Unlike the one prior comprehensive study on the topic (McClellan et al 2012 Environ. Res. Lett. 7 034019), we conclude that no existing aircraft design—even with extensive modifications—can reasonably fulfill this mission. However, we also conclude that developing a new, purpose-built high-altitude tanker with substantial payload capabilities would neither be technologically difficult nor prohibitively expensive. We calculate early-year costs of ~$1500 ton−1 of material deployed, resulting in average costs of ~$2.25 billion yr−1 over the first 15 years of deployment. We further calculate the number of flights at ~4000 in year one, linearly increasing by ~4000 yr−1. We conclude by arguing that, while cheap, such an aircraft-based program would unlikely be a secret, given the need for thousands of flights annually by airliner-sized aircraft operating from an international array of bases.